The current design is for the Arcanes to work independently of a set - but it's entirely possible that with upcoming balance changes, fixes, and feedback that the full 81 gear set may need a 3/3 or 6/6 Arcane 'set.' I don't think it'll need that because I think that breaking the Legendary 81 sets with individual Mythics and Arcanes will be a big boost over the full 81 6/6. We shall see, though. We shall see!
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